Methalloporphirins Catalyze Regio and Chemoselective Silylation of Hydroxy Groups with Hexamethyldisilazane (HMDS)

نویسندگان

  • Ali Reza Sardarian Department of Chemistry, Faculty of Science, Shiraz University, Postcode 71454, Shiraz, I.R. IRAN
  • Habib Firouzabadi Department of Chemistry, Faculty of Science, Shiraz University, Postcode 71454, Shiraz, I.R. IRAN
  • Shahram Tangestaninejad Department of Chemistry, Faculty of Science, Shiraz University, Postcode 71454, Shiraz, I.R. IRAN
  • Zohreh Khayat Department of Chemistry, Faculty of Science, Shiraz University, Postcode 71454, Shiraz, I.R. IRAN
چکیده مقاله:

Metalloporphirins; Cu(TPP), Mn(TPP)Cl, CO(TPP), Fe(TPP)Cl, zn(TPP) and Mn(OBP)Cl catalyze region and chemoselective silylation of hydroxyl groups with HMDS. Fe(TPP)Cl is the most effective catalyst and silylation occurs immediately in its presence at room temperature.

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منابع مشابه

methalloporphirins catalyze regio and chemoselective silylation of hydroxy groups with hexamethyldisilazane (hmds)

metalloporphirins; cu(tpp), mn(tpp)cl, co(tpp), fe(tpp)cl, zn(tpp) and mn(obp)cl catalyze region and chemoselective silylation of hydroxyl groups with hmds. fe(tpp)cl is the most effective catalyst and silylation occurs immediately in its presence at room temperature.

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Silylation of alcohols and phenols by HMDS in the presence of ionic liquid and silica-supported ionic liquids

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15 صفحه اول

Silylation of alcohols and phenols by HMDS in the presence of ionic liquid and silica-supported ionic liquids

In this research, different alcohols and phenols are subjected to the reaction with HMDS in the presence of ionic liquid and silica-supported catalysts. Silylation was accomplished under mild reaction conditions at room temperature in short reaction times and good to excellent yields.

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Silylation of Alcohols and Phenols Using HMDS Catalyzed by SiO2-Cl in Solution and Solvent-Free Conditions

Trimethylsilylation of a variety of alcohols and phenols, in the presence of silica chloride, using hexamethyldisilazane (HMDS) in solution and under solvent-free conditions is reported. Trimethylsilyl ethers were formed in excellent yields both for aliphatic alcohols and phenols without having an electron-withdrawing group. In addition, SiO2-Cl can be recovered and reused after drying.

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عنوان ژورنال

دوره 15  شماره 2

صفحات  54- 56

تاریخ انتشار 1996-12-01

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